In order to evaluate the impacts of LW contribution to aerosol radiative effects over East Asia,a dust longwave radiative parameterization scheme is integrated into the online mesoscale dust forecasting model GRAPES_CUACE/dust.A case modeling study shows that about half at surface and one third at TOA of the dust negative shortwave radiative forcing are cancelled by its positive longwave forcing over the dust affected area.In the dust layer,longwave radiation emitting by dust cools the atmosphere,which counteracts about 17%of shortwave heating of atmosphere during daytime and results in cooling of atmosphere simply during nighttime.At the same time,the atmosphere beyond the dust layer is warmed because of absorbing the LW radiation emitted by dust layer.Dust longwave contribution exerts more evident impact on the air temperature in lower atmosphere and surface.The surface air temperature cooling rate resulting from the dust solar radiation is cancelled about 40%by dust longwave warming at daytime.At nighttime,dust longwave contribution warms land and sea surface.The online calculation of dust LW radiation reduces about 15%relative errors of predicted AOD based on the dust model with only SW radiative feedback.This case study result suggests that dust longwave contribution has important impacts on the earth-atmosphere energy process,especially on the surface and in the lower atmosphere and should not be neglected in the study of dust radiation effects.
WANG HongSHI GuangYuZHU JingCHEN BinCHE HuiZhengZHAO TianLiang
Based on daily observation data at 222 meteorological stations in China,the characteristics of dust storms between 1997 and 2007 were examined.Next,the relationship between dust events and chlorophyll (Chl) a concentration in the Yellow Sea was investigated.There were six regions with high annual frequencies of dust storms.The seasonal distribution of dust storms showed spatiotemporal variation.The six regions with highest annual frequencies also exhibited high frequencies of dust storms in spring.Dust storms in most regions occurred in spring.Of all dust storms in China,sixty-five percent of all dust storms occurred during the spring.The area and frequency of dust storms were smaller in fall and winter than in spring and summer.A significant correlation was found between dust events and Chl a concentration in the Yellow Sea.High correlation regions included Qinghai-Xizang region,part of the Hexi Corridor,the western Inner Mongolia and Hetao Regions,and the Hunshandake Desert.The high correlation may be induced by the high ratio of dust storms in the abovementioned regions that arrive over the Yellow Sea,as inferred through a forward trajectory analysis;especially notable is dust transported at a lower altitude (< 3 km).
TAN Sai-Chun 1,2 and SHI Guang-Yu 1 1 State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029,China 2 Key Laboratory of Meteorological Disaster of Ministry of Education,Nanjing University of Information Science and Technology,Nanjing 210044,China
A Local Ensemble Transform Kalman Filter assimilation system has been implemented into an aerosol-coupled global nonhydrostatic model to simulate the aerosol mass concentration and aerosol optical properties of 3 desert sites(Ansai, Fukang, Shapotou) in northwestern China. One-month experiment results of April 2006 reveal that the data assimilation can correct the much overestimated aerosol surface mass concentration, and has a strong positive effect on the aerosol optical depth(AOD) simulation, improving agreement with observations. Improvement is limited with the?ngstr€om Exponent(AE) simulation, except for much improved correlation coefficient and model skill scores over the Ansai site. Better agreement of the AOD spatial distribution with the independent observations of Terra(Deep Blue) and Multi-angle Imaging Spectroradiometer(MISR) AODs is obtained by assimilating the Moderate Resolution Imaging Spectroradiometer(MODIS) AOD product, especially for regions with AODs lower than 0.30. This study confirms the usefulness of the remote sensing observations for the improvement of global aerosol modeling.
A large number of experimental and theoretical investigations of carbon dioxide （CO 2 ） spectra have been conducted since the most recent update of the High-Resolution Transmission Molecular Absorption （HITRAN） database. To maintain optimal parameters, the HITRAN 2004 CO 2 line list has been completely replaced by HITRAN 2008 data in the near-infrared region from 4300 cm-1 to 7000 cm-1 . To examine the effect of this change on the retrieval of CO 2 vertical column data from reflected sunlight spectra in the 1.61-μm spectral window, synthetic measurements for a given atmospheric state and instrument setup were generated and compared using radiative transfer model with the line-transition parameters from the HITRAN 2004 and 2008 databases. Simulated retrievals were then performed based on the optimal estimation retrieval theory. The results show that large systematic errors in atmospheric CO 2 column retrievals were induced by the differences in the HITRAN laboratory line parameters in the 1.61-μm region. The retrieved CO 2 columns were underestimated by 10 ppm using the HITRAN 2004 data, and improvements resulting from the use of the improved HITRAN database were more pronounced at a higher spectral resolution.
The line-transition parameters of the High Resolution Transmission （HITRAN） 2008 database have been updated relative to previous editions. The transmission spectra and sensitivity to changes in CO2 concentrations using line parameters from the HITRAN 2004 and HITRAN 2008 databases are compared to evaluate the effect of the database updates on retrievals of carbon dioxide vertical columns from nearinfrared reflected sunlight. This comparison is done in three spectral regions covering the 2.06-, 1.61-, and 1.58-μm CO2 bands used by the Greenhouse Gases Observatory Satellite （GOSAT） instrument and the planned successor to the Orbiting Carbon Observatory （OCO）. The updates to the HITRAN database have the largest effects on the transmittance and the off-line to on-line transmittance ratio in the 2.06-μm region and the smallest effects on these parameters in the 1.58-μm region. The influence of the updates to the HITRAN database on the off-line to on-line ratio calculation in the narrow spectral region 4855-4880 cm^-1 could be equivalent to a change in CO2 of more than 50 ppmv. Use of the HITRAN 2004 database will lead to an underestimate of the column CO2 abundance in the 2.06- and 1.61-pro spectral regions, whereas it will lead to an overestimate of the column CO2 abundance in the 1.58-μm spectral region.
