The magnetic properties of cobalt-based oxypnictides SmCoAsO are investigated by measuring magnetization,magnetoresistance and specific heat.The compound undergoes a ferromagnetic(FM) transition around Tc of 80 K,and a ferromagnetic to antiferromagnetic(AFM) transition below TN1 of about 45 K,and finally an AFM order of Sm ion at TN2 of 5.6 K.The weak FM order should originate from the itinerant 3d electrons of Co ions in the CoAs layers.We propose that the magnetic structure should be A-type AFM,which means that the FM order remains within the CoAs layer and the magnetic coupling between the CoAs layers becomes AFM below TN1 of 45 K.The AFM coupling between the CoAs layers should be very weak.A magnetic field μ0H of about 2 T may cause an AFM-FM metamagnetic transition.A rich magnetic phase diagram is established and the interplay between the 3d electrons of Co ions and 4f electrons of Sm ions is discussed.
LI YuKeTONG JunHAN HanZHANG LiTAO QianCAO GuangHanXU ZhuAn
This paper reports that high quality CuGeO3 single crystals were successfully grown by floating-zone technique and the magnetic property was studied. The temperature dependence of magnetic susceptibility below the spin-Peierls (SP) transition temperature (Tsp) under magnetic fields applying along both the a- and c-axis direction can be fitted well by a model of noninteracting dimmers. The spin gap derived from the fitting is consistent with other reports. There is a very weak anisotropy in the fitting parameters for different directions, which should be expected from a SP system. A small upturn in susceptibility at low temperature due to paramagnetic impurities and/or defects can be observed. A suppression of the upturn by magnetic field is first discovered in this system and the possible origins for this suppression are discussed.